Full metadata record
DC Field | Value | Language |
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dc.contributor.author | Hihath, Joshua | - |
dc.contributor.author | Bruot, Christopher | - |
dc.contributor.author | Nakamura, Hisao | - |
dc.contributor.author | Asai, Yoshihiro | - |
dc.contributor.author | Diez-Perez, Ismael | - |
dc.contributor.author | Lee, Youngu | - |
dc.contributor.author | Yu, Luping | - |
dc.contributor.author | Tao, Nongjian | - |
dc.date.available | 2017-07-11T07:01:29Z | - |
dc.date.created | 2017-04-10 | - |
dc.date.issued | 2011-10 | - |
dc.identifier.issn | 1936-0851 | - |
dc.identifier.uri | http://hdl.handle.net/20.500.11750/3433 | - |
dc.description.abstract | Designing, controlling, and understanding rectification behavior in molecular-scale devices has been a goal of the molecular electronics community for many years. Here we study the transport behavior of a single molecule diode, and its nonrectifying, symmetric counterpart at low temperatures, and at both low and high biases to help elucidate the electron-phonon interactions and transport mechanisms in the rectifying system. We find that the onset of current rectification occurs at low biases, indicating a significant change in the elastic transport pathway. However, the peaks in the inelastic electron tunneling (IET) spectrum are antisymmetric about zero bias and show no significant changes in energy or intensity in the forward or reverse bias directions, indicating that despite the change in the elastic transmission probability there is little impact on the inelastic pathway. These results agree with first principles calculations performed to evaluate the IETS, which also allow us to identify which modes are active in the single molecule junction. © 2011 American Chemical Society. | - |
dc.publisher | American Chemical Society | - |
dc.title | Inelastic Transport and Low-Bias Rectification in a Single-Molecule Diode | - |
dc.type | Article | - |
dc.identifier.doi | 10.1021/nn2030644 | - |
dc.identifier.wosid | 000296208700088 | - |
dc.identifier.scopusid | 2-s2.0-80055015815 | - |
dc.identifier.bibliographicCitation | ACS Nano, v.5, no.10, pp.8331 - 8339 | - |
dc.subject.keywordAuthor | molecular electronics | - |
dc.subject.keywordAuthor | STM-break junction | - |
dc.subject.keywordAuthor | Inelastic electron tunneling spectroscopy | - |
dc.subject.keywordAuthor | IETS | - |
dc.subject.keywordAuthor | single-molecule conductance | - |
dc.subject.keywordPlus | 1ST-PRINCIPLES | - |
dc.subject.keywordPlus | Anti-Symmetric | - |
dc.subject.keywordPlus | Article | - |
dc.subject.keywordPlus | Behavioral Research | - |
dc.subject.keywordPlus | Chemistry | - |
dc.subject.keywordPlus | Distillation | - |
dc.subject.keywordPlus | Elastic Transmissions | - |
dc.subject.keywordPlus | Elasticity | - |
dc.subject.keywordPlus | Electric Conductivity | - |
dc.subject.keywordPlus | Electric Rectifiers | - |
dc.subject.keywordPlus | Electrical Equipment | - |
dc.subject.keywordPlus | Electrical Equipment and Supplies | - |
dc.subject.keywordPlus | Electrode | - |
dc.subject.keywordPlus | Electrodes | - |
dc.subject.keywordPlus | Electron | - |
dc.subject.keywordPlus | Electron-Phonon Interactions | - |
dc.subject.keywordPlus | ELECTRON-TUNNELING SPECTROSCOPY | - |
dc.subject.keywordPlus | Electron Tunneling | - |
dc.subject.keywordPlus | Electrons | - |
dc.subject.keywordPlus | Equipment Design | - |
dc.subject.keywordPlus | First-Principles Calculation | - |
dc.subject.keywordPlus | IETS | - |
dc.subject.keywordPlus | Inelastic Electron Tunneling | - |
dc.subject.keywordPlus | Inelastic Electron Tunneling Spectroscopy | - |
dc.subject.keywordPlus | JUNCTIONS | - |
dc.subject.keywordPlus | Low Bias | - |
dc.subject.keywordPlus | Low Temperatures | - |
dc.subject.keywordPlus | METAL | - |
dc.subject.keywordPlus | Molecular-Scale Devices | - |
dc.subject.keywordPlus | Molecular Electronics | - |
dc.subject.keywordPlus | Molecules | - |
dc.subject.keywordPlus | Phonon | - |
dc.subject.keywordPlus | Phonons | - |
dc.subject.keywordPlus | Pyrimidine | - |
dc.subject.keywordPlus | Pyrimidine Derivative | - |
dc.subject.keywordPlus | Pyrimidines | - |
dc.subject.keywordPlus | Rectification Behavior | - |
dc.subject.keywordPlus | Reverse Bias | - |
dc.subject.keywordPlus | Scanning Tunneling Microscopy | - |
dc.subject.keywordPlus | Single-Molecule | - |
dc.subject.keywordPlus | Single-Molecule Conductance | - |
dc.subject.keywordPlus | Single-Molecule Junctions | - |
dc.subject.keywordPlus | Single Molecule Diodes | - |
dc.subject.keywordPlus | SPECTROSCOPY | - |
dc.subject.keywordPlus | STM-Break Junction | - |
dc.subject.keywordPlus | SUBSTITUTION | - |
dc.subject.keywordPlus | Sulfhydryl Compounds | - |
dc.subject.keywordPlus | TemPERATURE | - |
dc.subject.keywordPlus | THIOL | - |
dc.subject.keywordPlus | Thiol Derivative | - |
dc.subject.keywordPlus | Transport Behavior | - |
dc.subject.keywordPlus | Transport Mechanism | - |
dc.subject.keywordPlus | Transport Pathways | - |
dc.subject.keywordPlus | UNIMOLECULAR RECTIFIERS | - |
dc.subject.keywordPlus | VIBRATION SPECTRA | - |
dc.subject.keywordPlus | Zero Bias | - |
dc.citation.endPage | 8339 | - |
dc.citation.number | 10 | - |
dc.citation.startPage | 8331 | - |
dc.citation.title | ACS Nano | - |
dc.citation.volume | 5 | - |
dc.description.journalRegisteredClass | scie | - |
dc.description.journalRegisteredClass | scopus | - |
dc.relation.journalResearchArea | Chemistry; Science & Technology - Other Topics; Materials Science | - |
dc.relation.journalWebOfScienceCategory | Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary | - |
dc.type.docType | Article | - |
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